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SUMMARY:Probing electronic processes in molecular complexes by coherent mu
 ltidimensional visible\, UV and X‐Ray spectroscopy
DTSTART:20120604T121500
DTSTAMP:20260407T210946Z
UID:ed3f88d25181e202b7dc1b8f0a6e2da010f81191e78022475fb7ee68
CATEGORIES:Conferences - Seminars
DESCRIPTION:Shaul Mukamel\, Department of Chemistry\, University of Califo
 rnia\, Irvine\, Irvine\, California 92697‐2025\, USA\nEnergy‐ transfer
  and charge‐separation pathways in the bacterial reaction center may be 
 revealed by coherent two‐dimensional optical spectroscopy. The excited s
 tate dynamics and relaxation of electrons and holes are simulated using a 
 two‐band tight‐binding model. The dissipative exciton and charge carri
 er motions are calculated using a transport theory\, which includes a stro
 ng coupling to a harmonic bath with experimentally determined spectral den
 sity\, and reduces to the Redfield\, the Förster\, and the Marcus express
 ions in the proper parameter regimes. Direct spectroscopic signatures of t
 he charge separation are identified.
LOCATION:CE 1 3 https://plan.epfl.ch/?room==CE%201%203
STATUS:CONFIRMED
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